21 Sermons/lectures, 2 letters, and a published inaugural discourse by Rev. Isaac Anderson, D.D.

Seven letters, two poems, one sermon outline, Presbyterian Witness publishing proposal, and other material created by or pertaining to the family of Andrew and Ann Elizabeth (Gillespy) Blackburn.

Two essays written in 1922-1923 by MC Freshman Robert Wilson Bishop (class of 1926) titled "My First Twenty-Four Hours in Maryville" and "What My First Semester in College Has Meant to Me."

Diplomas, photographs, programs, and invitations collected by James Morrison Brown during his time as a student at Maryville College.

Typewritten copy and extracts of 1880 Autobiography of Rev. William E. Caldwell (MC class of 1848) and obituary of Mrs. Mary Thompson Anderson Caldwell.

Speeches, correspondence, clippings, photos, two photograph scrapbooks, and other material created by or pertaining to US Consul General Edwin Sheddan Cunningham.

Song lyrics, musical transcriptions, interview notes, scrapbooks, publications, and other material created by the Dr. Dorothy Horne and Oliver Hamby ballad project in 1937-1938.

Original unpublished music composition manuscripts and published books by Dr. James H. Laster.

21 letters from Rev. Robert Henderson DD (Presbyterian minister) to Col. Francis A. Ramsey of Swan Pond (now known as Ramsey House in Knoxville, TN) from 1807-1820.

Three diaries covering 1847, 1852, and 1855-1857 of Maryville College student and alumnus Jonathan Maxwell Hoffmeister [Huffmaster] (class of 1848). 1847 Diary contains descriptions of classes, students, faculty, local community, and family members (including deaths of brother and fiancee in local epidemic). 1852 and 1855-1857 diaries cover family life and ministry in northeast Tennessee.